I would look at a cylinder table, maybe like this one Scuba Cylinder Specification Chart from Huron Scuba, Ann Arbor Michigan and compare the buoyancy characteristics of the HP and LP tanks you are considering, might have an effect on your weighting.
Also, my regulators are older yoke mount and only rated for 3000psi service, so I probably wouldn't fill an HP tank to over 3000psi.
Also, my regulators are older yoke mount and only rated for 3000psi service, so I probably wouldn't fill an HP tank to over 3000psi.