Depends on what you want to do with them. I see on your profile you have 0-24 logged dives. Why do you want such a big tank? Are you concerned with your air consumption? I can tell you, as an instructor, it get's better after about 30 dives.
As far as High pressure tanks go, it really doesn't matter weather it's HP or LP. 120 cf is 120 cf no matter how small a space you pack it into. Which leads to another point. 120's are long. If you're short, this may be a problem for you. Also, if you're diving a 120 and your buddy has an aluminum 80, what are you going to do with all the extra air when he has to come up?
Steel tanks are more negatively buoyant than aluminum tanks. Many divers, including me, prefer this. As far as doubles go, there are training issues which you need to address. You shouldn't just throw on a set of doubles and go diving. There are equipment configuration issues and redundant systems to consider. Most agencies won't train you to TEC dive or use doubles before you have 100 dives, 10 nitrox dives below 100ft. and a rescue diver certification.
Bottom line, if you want a steel tank, get an 80 cf. for now. Later, you can always sell it when you upgrade.
Hope this helps.