@DiveTucson's proposition makes a lot of sense. It is a streamlined setup that yields a significant bailout volume plus an easy access to a DPV. If the overall height - chestmout CCR + doubles - are not a concern for the dive, then why not?
A twinset of a single gas could make sense on say a Mod1 or Mod2 dive, where that one gas can basically just be your bottom gas, and it gets you easily up to that first deco gas (stated as 50%) with no real compromises on ppO2, END, or deco.
You could just do the whole dive as an OC dive if you had to, because you brought so much bottom gas. And you already are a twinset diver. But you wanted to CCR instead, because of numerous advantages, so you add on a chestmount CCR.
I'm with you!
That said, you probably could have done exactly the same thing with just a single cylinder of bottom gas on your back, or the deep and deco gases sidemounted, with nothing on your back.
The twinset of bailout approach sounds pretty much the same as the GUE/DIR(?) approach of putting the bottom gas on your back as a mini twinset, so that you don't have to carry it as a stage cylinder. But this is a bottom gas.
However, once you are going to Mod3 depths (e.g. ~100 metres), there is no single 'back gas' that is going to work at the bottom, and also be ideal as a travel gas all the way up to 20 metres (the 50%, in examples given). A proposed solution earlier was to just tag on a new extra stage cylinder of deeper gas. It is easy to see how this was chosen as a simple fix for going deeper.
Unfortunately, now you are carrying a twinset of gas that used to be your Mod2 bottom gas, but is now just some kind of travel gas. And that is no longer efficient. There is no longer much justification for that extra cylinder of travel gas. You'd actually be better off with another cylinder of deeper deco gas--for example, the 32/20 that I explained in the previous example.
So we could just keep adding on cylinders, or else staging them along the way for later retrieval. I guess that is fine.
But if we are talking about what is ideal, or trying to limit the number of cylinders involved, then the twinset travel gas approach raises eyebrows from a gas planning perspective. I guess you could argue that the twinset is a mini twinset, but I am not convinced this is any better than a single full sized cylinder.
The love for manifolded twinsets is gospel in open circuit tec courses, it is a true symbol of tec. The holy 'valve drill' is like praying to the tec gods. But I've not heard of a single person ever actually needing it on a real dive. Not in recent times.
Granted, there could be other reasons why you want all that double share of extra mid-depth gas, like if you think it's possible that you could get delayed from leaving the top of a wreck, or your cave exit is at a certain depth, etc.