From what I remember, Aluminum was chosen primarily to save weight for a fly-away package. The strange part is the design wasn't very friendly to aircraft loadmasters. Most portable chambers have skids and several places to attach slings to make them crane and forklift-friendly. This image also shows how ergonomics have improved.
They were also pretty concerned over chamber fire safety in those days and Aluminum was desirable because a dropped tool won't spark. That is one reason that all deck plates in modern chambers are Aluminum now.
Edit:
1969-73