The leak is from the isolator valve, not the crossbar.
This leak would allow both cylinders to drain. If both cylinder valves were open, then both cylinders would drain equally through the leak.
However, if one of the cylinder valves were closed, then such a leak would drain only the cylinder with the open valve.
Hmmmm? Seems to me the isolator is working fine. He closed it and it saved the gas in the tank that has no leak while the leaky tank is draining....exactly what the iso valve is supposed to do. Or did I read something wrong?
Anyhow, getting back to the valves, the o-rings in the valve are likely all downstream of the valve seat itself, so the most likely thing is the burst disc or the tank neck o-ring. In fact, that's all it could be unless you have a leaky valve seat, which is pretty rare. One other possibility is a leak on the manifold crossbar, but those usually have 3 o-rings in series, so it's almost unheard of to have a leak there.
If you want to eliminate the possibility of a leaking valve seat, just put a regulator that you know does not leak on the post, then store the tanks for a while with that post open (iso still closed) and see what happens. If the leak stops, the problem was the valve seat, if not, burst disc (probably), tank neck o-ring (maybe a bit less likely) or crossbar. (very unlikely.)
If it were my doubles, probably first thing I'd do is drain the offending tank, replace the burst disc, open the iso to equalize, then close it and store, check back in a few days. No more leak? Off you go....
All the other fixes require dismantling the doubles, and at that point I would agree that it's time to rebuild the valves.
Edit: looks like you probably already took care of it.