The Kraken:
One thing that I do want to incorporate in the doubles set up is the ability to use a single tank to accompany my wife on recreational dives...
You should set up your own doubles, preferably with the help of an experienced buddy or the shop where you bought the bands and manifold, etc. Inspect your tanks yourself. You'll soon see that its a pain in the butt to get them set up exactly right. Once done, you don't want to be pulling them apart all the time. Get them right then leave them alone. If you want to dive with your wife who is wearing a single cylinder, have at it - but do so in your doubles. Getting used to them, the valve drills, the trim, the whole thing, requires lots of practice. If you're transitioning, plan to dive in them all the time. (Which is another reason not to get a set of heavy-as-hell steel pigs that you have to hump all over.)
I'm a tad concerned about the positive buoyancy characteristics of the Al 80's as I'm still diving wet.
Then get neutrally bouyant aluminum 80s. Luxfer makes some nice ones. Thicker walls, so heavier, pumped to 3300 psi. I have a set of these, and they are excellent tanks. Remember also that you weight yourself to trim out with your doubles empty. There are many options. I use a 10lb Halcyon V-weight with my aluminum doubles (and a 6lb backplate), with my sets of 130s I simply leave off the V-weight. You can use trim weights, channel weights, plates that bolt to your backplate (Tobin has some nice ones), etc. - but you'll weight yourself to trim out empty. No worries on that end. Its just that in a wetsuit you'll be heavy on the front end of the dive (when it compresses at depth), thus need more gas in your wing, thus more drag, thus more energy, etc. etc. You want to think about the front end, not the back end.
I've been eyeballing the PST HP 80's and 119's.
Try'em before you buy'em. 119s are not bad tanks, but could get interesting in the ocean in a wetsuit. I owned a set of these. They stood me on my head. I went to 130s. Much better. Depends on many factors. Best is to borrow different sets and try them out in an open water setting. Generally speaking, get a drysuit BEFORE you buy steel tanks. Why? Because the drysuit you buy and the undergarment you select plays a huge role in how the tanks trim out on you in the water. Its a system. The parts all have to work together.
FWIW