There was an extended discussion on another forum about a very deep dive (180 meters) on which the diver got seriously bent. The diver posted the details of his dive so that there could be an extended discussion about it. He had used the philosophy of doing the deepest ascents faster than the shallower ascents, just as you describe. There is nothing inherently wrong with this approach--it makes sense, in fact.
As I recall the discussion, the consensus was, however, that his dive plan from decompression software assumed a steady 9m ascent rate. In shallow decompression dives, it would make little difference, but on a dive as deep as that, it made a big difference. The plan's first stop assumed he had spent a certain amount of time ascending (and off-gassing). If you input his actual ascent rate, the software calls for the first stop to be deeper.
You can see a similar issue with people following decompression software plans on deep dives when they descend faster than the software is set for. Let's say you plan a dive to 90 meters/300 feet, and the software has a 15 meter/50 foot per minute descent rate. You are planning 20 minutes before beginning the ascent. You instead descend at 30 meters/100 feet per minute. (These are not random or unrealistic numbers--I had this discussion with someone who loved to do rapid descents like that, without adjusting his planned ascent profile.) At the planned descent rate, it takes 6 minutes to reach the bottom. At your actual rate, it takes 3 minutes to reach the bottom. At the planned rate, your first 6 minutes of diving were at an average depth of 45 meters/150 feet. At the actual rate, your first first 6 minutes were at an average depth of 70 meters/225 feet. That will make a significant difference in the dive profile.