Here's why I say stroke crap.
What's the most common cause of death in technical diving? Improper gas switches. This dive plan already has 4 different gases for what is effectively a short bounce dive. Every time you add an extra gas switch you are increasing the complexity and the chances of screwing up, so try to maximize the utility of the gases and minimize the gas switches (I like doing a gas switch no more frequently than once every 5 stop depths).
We might then ask "why does he want to use 80%"? You wrote:
What's everyone's thoughts on EAN80 vs. 100% O2? In light of the plan outlined above, EAN80 would obviously lower OTU's and CNS% and reduce the need for air-breaks whilst only increasing the total runtime by 3 minutes (i.e. a runtime of 106 minutes as opposed to 103 minutes).
Now adding 80% doesn't really buy you much in terms of benefit for this dive plan. In terms of lowering your OTU's and CNS%, your CNS clock is only going to be on the order of 60-70% from the original dive plan if you use 100% oxygen to begin with and at 9m 80% has a PO2 of 1.6 (just like 100% is at 20'). All this while you're reducing the usefulness of your 50% gas and introducing an earlier gas switch.
Additionally, the first proper first aid for DCS is 100% oxygen -- you should ALWAYS have oxygen available for you on days you do 100m dives. Heck, I usually keep an extra bottle of oxygen "for the drive home" in case stuff goes wrong.
Finally, AJ hinted at this but I had missed it until this morning because of the metric to imperial conversions. Your plan to add 80% is because you're here worrying to hell about CNS and OTU's but you're completely missing the boat on having enough bottom mix to do the dive safely. 2x12L cylinders are pretty small, for those of us on this side of the pond that's basically LP77's.
A CNS clock of 70% is not going to mean you will die from oxygen toxicity. 130 OTU's on a dive is not going to mean you will get pulmonary oxygen toxicity. Running out of gas does mean you will likely drown.
You're worrying about the wrong things, and that's why I said "stroke crap."